After moving to Los Angeles, Hallett worked as a Runner for an agency and then as a property manager. He eventually became a personal assistant to Kai Cole, wife of Buffy the Vampire Slayer creator Joss Whedon. When the couple and their friends saw Hallett singing at the "B.B. Kings" lounge at Universal CityWalk, Whedon conceived a new character for his new show Angel: Lorne, an anagogic demon who reads the hearts and futures of his guests as they sing in his karaoke bar. Hallett was invited to try out for the part, and won it after three auditions. Angel was his first real job as an actor, though he did play an extra role in a 1999 episode of Buffy; he acquired agent Pat Brady only after she spotted him singing and acting in "Judgment", the premiere episode of Angel's second season.