A member of the Actors Studio, Sands' performance in the Studio's 1964 production of James Baldwin's Blues for Mr. Charlie was a highlight of that show, and one which would be sorely missed during its subsequent London engagement when Sands had already committed to co-starring with Alan Alda in the original Broadway production of The Owl and the Pussycat (1964) for which she was nominated for a Tony Award for Best Actress in a Leading Role. Sands was sought eight years later to provide a track for the Original New York Cast album of Free to Be... You and Me. Unfortunately, she had died by the time the ABC Afterschool Special had begun production and her previously recorded vocal track was not selected for inclusion. In 1970, Sands co-starred in the film The Landlord, and then appeared in Doctors' Wives and Georgia, Georgia. In his memoirs, Bob Dylan tells of meeting Ms. Sands at a party and states that she was, "an electrifying Actress who I might have been secretly in love with ..."