Larry Lee Simms worked as a child model from the age of two years and was discovered by a Hollywood talent scout when he appeared in a 1937 Saturday Evening Post advertisement. His first film for Hollywood was The Last Gangster (1937), where he played Edward G. Robinson's young son. Simms got well-known with his appearances as Alexander "Baby Dumpling" Bumstead in the popular Blondie film series starring Penny Singleton. Between 1938 and the end of the series in 1950, Simms appeared as Alexander in 28 films of the Blondie comedies and was a regular cast member. The child actor earned at one time $750 a week. In 1946, Simms joined the cast of the Blondie radio program, portraying Alexander there as he had in movies.