In 1967, he teamed up with flautist Hariprasad Chaurasia and Guitarist Brij Bhushan Kabra to produce a concept album, Call of the Valley (1967), which turned out to be one of Indian classical music's greatest hits. He has composed music for many Hindi films in collaboration with Hariprasad Chaurasia starting with Silsila (1980). They came to be known as the Shiv-Hari music duo. Some of the movies they composed music for were big musical hits, such as Faasle (1985), Chandni (1989), Lamhe (1991), and Darr (1993).